Hurt them in the spine really hard
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No, you can't. If you want to paralyze a Pokemon, it has to be awake.
Here are two Pokemon Moves that can Paralyze Pokemon: Shock Wave and sometimes Body Slam.
put them to sleep, or paralyze them
Simple either Do the special conditions like poison,paralyze, sleep and I say that you paralyze it and make it fall asleep and use a dusk ball or you could use the master ball that Cyrus gave you and you have caught a Giratina
you have to weaken it to like no life and then you have to paralyze it and use ultra balls