Kyruem is pretty hard to catch unless you didn't use your Master ball to catch Zekrom, I caught Zekrom with a Quick ball.
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A Pokemon's catch rate can range from 3 (hardest to catch) to 255 (easiest to catch). Hardest to catch (catch rate = 3): - Uxie - Mesprit - Azelf - Heatran - Regigigas - Giratina - Cresselia - Manaphy - Darkrai - Arceus Easier to catch (catch rate = 30): - Dialga (& Palkia) Easiest Sinnoh legendary to catch (catch rate = 45): - Shaymin
You can't catch it in Black, but you can catch it in White. In the White Forest.
Not including the legendaries and special pokemon ( ones that you can only catch once ) feebas is the hardest and rarest pokemon to catch
You can not catch any of them in black or white, but I think that you can catch all 3 in diamond.
white forest