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You need to do the "Trouble on the Homefront" quest, anytime 'after' you complete Project purity, you need to get yourself within Radio reception distance of Vault 101, Megaton for instance, and you will hear the Vault 101 distress signal on you Radio, listen to it and you will then know what to do.

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Q: When can you get back into vault 101 in the game Fallout 3?
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