Surf From New Bark Town To Kanto Then Go Through The Cave. After Go Up To Victory Road. From there go through And You Will arrive at the indagoplaato: Pokemon league!
Good Luck Victory Road Is A Little Tough.
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Mt. Silver or the Pokemon league
You can defeat the Pokemon League by defeating the Elite Four and the Champion in Pokemon Soul Silver.
In Pokemon Heartgold you need Ho-Oh before going to the Elite Four/Pokemon League so I am sure it's the same for Pokemon Soulsilver.
you have to beat the Pokemon league then go to the Pokemon transfer lab at route 15 you need to go onto ds download play to transfer Pokemon from silver to white but you cannot transfer Pokemon to soul silver
Usually ultra balls are sold in the later cities try blackthorn city or the Pokemon league.