You have to enter Mt. Coronet through Route 207, and go with good pokemon, because you battle Mars and Jupiter, then Cyrus, then you battle and try to capture Palkia. (Hint: Use the Master Ball Cyrus gave you. You don't even have to hurt it.)
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No, but skitty can be caught on route 222 in Pokemon diamond pearl and platinum
Defeat Team Galactic on Mt. Coronet.
route 222
swarms on route 222
pokeradar on route 222