Jiraiya fights Pain/Pein from episodes 126-133 BUT IF YOU WANT JUST THE FIGHT WITHOUT THE INTRO WATCH EPISODES (watch 129 if u want to watch konan fight too) 130-133
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The pony-tail Pain. He was a ninja that fought Jiraiya during his journey for his disciple. His body was used by Nagato years later as the first Animal Path. In the anime, the character Naruto's fight with the ninja in Jiraiya's story is slightly based off Jiraiya's fight with this Fūma ninja.
I think it's episode 94. It's when orochimaru, tsunade, and jiraiya fight at the same time. kabuto tries to stab naruto, but he grabs his arm, has his clone make the rasengan, and hits him with it =)
Episode 190 in naruto,pre-shippuden,but still in the first naruto series. It's in the filler episodes
I think it's episode 107 or around it.
No episodes exist of naruto training with jiraiya as that 3 years in the story was the transition from naruto to naruto shippuden. Some flashbacks of the training are shown during the first couple of episodes of shippuden