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when he is insanely low - less than 1/4 cm of hp

At any time--the catching of Azelf comes mostly down to luck. For example, I currently have Azelf down to one HP and asleep; however, I have used fifty five dusk balls and still he continues to break free. This is because Azelf has a 3% Catch Rate out of a hundred, which is low enough to send people to mental institutions. It is highly unlikely lowering its HP amounts to making up for the remaining 97%. For all intents and purposes, catching Azelf is more up to chance than timing or HP lowering. That's not to say don't do it; just take the advice with a grain of salt.

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12y ago

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Q: When do you use a dusk ball to catch azelf?
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