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I used a Master Ball to catch Palkia, but that was before I knew Uxie, Azelf, and Mesprit were legendary.

It all depends on the types of the Pokemon or how long you expect the battle to last.

For Water-type or Bug-type legendaries, use Net Balls.

For long-lasting battles, use a Timer Ball.

For cave or night battles, use a Dusk Ball. (I recommend this for the Generation IV legendary trio, Uxie, Azelf, and Mesprit.)

For Water-types, use a Dive Ball. (I'm not sure where you get this.)

An overall ball to use would be the Ultra Ball.

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15y ago

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Q: What poke balls do you use to capture legendary Pokemon?
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