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Yes, the Ultra Ball has a 4x catch rate than a Premier Ball, which has the same catch rate as a normal Poke Ball. It is commonly used to catch rare or Legendary Pokemon.
The Ultra Ball is the ball with the highest catch rate after the Master Ball.
The only way to have a 100% catch rate is to use a Master Ball.
Darkrai can be caught in any kind of Poke Ball, but Ultra Ball has 4x the catch rate by itself, which is pretty high.
Net Balls are highly recommended, since they have a high catch rate on Bug or Water Types. I caught mine with a Heal Ball, though I was extremely lucky since Balls with a 1.0 cath rate have a 0.5 catch rate if used against legendaries...