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the best way is to get faster pokmeon (faster then the entei and raikou) i recomend a high level raichu and a high level gengar

first pralyze the Pokemon using thunder wave in raichu then they are going to flee

the second time you hunt them doen have gengar in front of your party when the battle begins use the move mean look then the entei or raiku whont be abel to escape (note if you switch out gengar mean look whont work) with gengar make them go to red health and start throwing pokeballs (i recomend searching the legendary dogs at night because dusk balls are more effective at night)

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Q: What is the best way to catch Raikou and Entei in Pokemon HeartGold?
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