You can not breed legendary pokemon.
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Raikou is best because entei and suicune are fegget Raikou all the way 2 reasons He is way cooler then Entei and Suicune. Number 2 he could whoop Suicune and Entei in a battle So suicune and entei are good but overall raikou is better
Starter:Charmander-Suicune Squirtle-Raikou Bulbasaur-Entei
Entei, Suicune, and Raikou are not available in Pokemon Emerald, Ruby or Sapphire. They can be brought into the game by trading.
Entei because it learns eruption and fire blast! Hope that heps!
Suicune is not on Fire Red, Suicune is only found in Silver, Crystal and Gold versions. Suicune is one of the 3 Legendary Dogs, Entei, Suicune, and Raikou. Once killed the Legendary Dogs are gone forever, so it is important to capture them. They will be a great adaptation to your team.