The level 83 cockroach soldiers drop them on occasions in runescape, for nonmembers and members.
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Greater demons drop Rune Full Helms and Rune KitesLesser demons drop Rune Med Helms (Rune Helms)Cockroaches drop Rune Square Shields and Scimitars
Fire Giant's tend to occasionally drop Rune Battle axes.
Of couse!If your asking about nonmember monsters, then there is the level 83 lesser demon that has a rare rune medium helmet drop. There is the level 82 Cockroach Soldier that has a rare drop of a rune scimitar or a rune kiteshield. It also rarely drops runite ore. Greater demons also drop rune items: they are found at the demonic ruins and in the Wilderness Volcano.For more info check out the RuneScape wikia website.
The quest "Rune Mysteries" is a prerequisite to mine rune essence, and to make the actual runes.There is a rune essence mine. Go to Aubury (south of the eastern Varrock bank); he will teleport you if you did the quest.You can of course buy rune essence from the Grand Exchange - rune essence that was obtained and sold by other players.You also get small amounts of rune essence as drops from certain monsters.
Rune Med-Helmet.