Well some Pokemon you will have to evolve the easiest way to get 60 Pokemon is to train Pokemon that evolve quickly or catch Pokemon that evolve by evolution stone like clefairy, nidorino, nidorina, jigglypuff, weepinbell, gloom, growlithe, vulpix, pikachu, evee, exeggcute. Trading helps too.
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The only way to get it is by the safari zone which makes it harder to catch it there really is no easy way to get it so when you find it i suggest trying to capture it as soon as you find it.
EASY!!!!!!!!!!!!!!!!!!!!!!! you catch near the start of the game.
Two ways Easy way: Migrate from FireRed/LeafGreen (Recieve at Lv 25 in Silph Co.) No-Trading Way: Can be found in the Post-Dex area in Victory Road in the Water.
You use block or mean look at a lengedary Pokemon and then make it asleep and weaken it. After that, it's pretty easy to catch it. If you wanna catch LUGIA then you weaken it, lure it to sleep, and then it's easy to catch. Pokeballs and ultraballs are good against legendarys.