I'm not really sure about this. Maybe you can use GameShark. It's the best recommended game hacker. I have NO idea how to use it, so here's an example. It might be the wrong way though. Let's say you have GameShark. Your playing Pokemon Platinum and you're confronting a lvl 100 Giratina. You go and get ur GameShark and use it on your DS.
Then, as you use it, you program it to make normal Pokeballs never fail at catching Pokemon. People also talk about catching a Mewtwo in a normal Pokeball.
I know a different Pokeball that you probably know about, the Masterball. Only one per game. There's a hack to get multiple groups of 99 Masterballs in ur bag, but I don't know it. It's for GameShark, so you can search on the web.
Hope you figure out all this confusing information!
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Poke-mart.
get a gamboy action replay and find the cheat on the computer
weaken it's health to red and paralyze it. use tons of pokeballs or other kinds.
You get the red shard from the red garados if you fail to catch it at the lakeof rage.
You can't get premier balls in Fire Red, a lot of peope say you can get it by purchasing at least 10 pokeballs at the pokemart but it does't work in Fire Red. Sorry