Open up the Crafting Table space and use Leather, Iron Ingots, Gold Ingots, or Diamonds to make this set of armor:
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iron diamond gold and leather
There is no way to make zombies wear leather armor, but sometimes zombies can naturally spawn already wearing the armor.
Helmet, chest plate, leggings, and boots.
The best armor in that mod is Halite armor.
Diamond armor is definitely the best armor in minecraft. It protects you the most and last for a really long time.