u can find it in tin tower after saving radio station of golden rod city from team rocket..
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You can get lugia, ho oh, entei, suicune and raikou
the legendaries available in Crystal is Raikou, Entei and Suicune. Lugia and Ho-oh are available too.
suicune is top legendary dog just play Pokemon crystal and you'll see.
The most important pokemon to catch in any game is its mascot, in this case Suicune.