You might be thinking of Shirley Manson - she also played Catherine Weaver, and she sung Samson and Delilah in Season 2 Series 1
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It's Pie Jesu sung by Sarah Brightman
"In Finding You, I Found Love"
The song "Angel", which is often mistakenly called "In the Arms of an Angel" is sung by Sarah Machlan. The song first appeared on Sarah's 1997 album "Surfacing" and peaked at number four on the Billboard charts. The song is about the Smashing Pumpkins keyboard player, Jonathan Melvoin who overdosed on heroin and died in 1996.
Gene sings the song "uso".
who sings the song let me know