In The Flintstones episode "The Twitch", Hal Smith did the speaking voice for 'Rock Roll'.
For the 'Bedrock Twitch' song, though, I thinkthat Glen Campbell sang and played guitar, although it was uncredited.
It sounds like Campbell's voice, and he was both a solo artist on Capitol Records and a member of Hal Blaine's 'Wrecking Crew' (studio musicians) in 1962, when the episode was made, so it's entirely possible that the Wrecking Crew got the studio call, and Campbell was tapped to do the vocal and guitar parts, although I can't confirm it...
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Tom Jones sang the song.
Who sang the last song from the movie in Black Rain?
Michael Jackson sang the song "Blue Gangsta."
Agustin Lara first sang this song in 1932
Bill Kaulitz sang the song. It is performed by his band Tokyo Hotel