In Naruto Episode 52: Ebisu Returns: Naruto's Toughest Training Yet!
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The episode of Naruto when Jiraya dies is in the 133rd episode of the series. The name of the episode was The Tale of Jiraiya.
He masters it in Naruto Episode 53- Long Time No See: Jiraya Returns!
Naruto episode 216
Actually, he does meet naruto in episode 12 and they battled in episode 14-15 or somewhere near that.
episode 58 its really naruto shippuuden episode 58!