Let Me Sign by Robert Pattinson. It's available on iTunes but only as 'Album Only'.
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Eyes on Fire by Blue Foundation
yes, Robert Pattinson plays the piano in real life
The song playing in the ballet studio in Twilight when Edward is sucking the James' venom out of Bella's blood is Let Me Sign by Robert Pattinson, who plays Edward in Twilight and New Moon.
The Twilight Saga
The twilight scene song is "Flightless Bird, American Mouth" by Iron&Wine