They first appeared in episode 7 then they went to the human world and they appeard again in episode 14
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Hiro appears in the Soul Eater in Season 1 Episode 32.
Bart sells his soul in the aptly titled Season Seven episode, Bart Sells His Soul
Episode 1, will soul eater become a death scythe and episode 4, a remedial lesson in the .
episode 157
There is an episode towards the end when everyone starts fighting Asura and I recall Soul holding her then, but not really.