Yes I do believe buster bunny was in love with babs. Babs was always around him and sometimes he would get tongue tied. She seemed like a good match for him also.
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In the show "Tiny Toon Adventures," Buster Bunny and Babs Bunny are close friends and partners, but their relationship is platonic. They share a strong friendship and work well together to create entertaining and humorous adventures. There is no indication that Buster is in love with Babs romantically.