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Plug your iPod into your computer and open iTunes. On side menu of iTunes you will see an iPod symbol (this is under Devices, the third category down). Click on the iPod symbol and scroll down to the third category, Options. Click on SYNC ONLY CHECKED SONGS AND VIDEOS. Then go to your iTunes library and un-check all of the songs and/or videos that you do not want on your iPod. This will allow you to keep your iTunes music, but it will take it off your iPod.

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Q: How do you delete music from iPod but not from iPod library?
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