The way to delete a Smule account is to delete the application from the android or iPhone device. There are several different applications the Smule owns. It would depend on which application for the proper way on how to delete just one account.
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To delete an app put your finger on the app for awhile and then the apps should start wiggling or shaking. Then press the x buttom on the app.
In Itunes itself, just press the delete key. If you want to delete from the iPod itself, call up the contents when it is plugged in, highlight (by clicking) what you want to delete, then press the delete key. Alternatively, just delete it from Itunes then sync your iPod - it will cope exactly what is in iTunes.
You can delete them the same as deleting a tagged song. Simply rub to the right on the song/tag, it brings up a red delete at the right which you can then delete with
you can delete your music library from the advanced options
Click on the Photo Album you want to delete. The Click "Edit Photos." There should be a series of tabs, and one of them should say delete. That is where you can delete all photos from the album. This deleted the album and all contents.