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By area, the largest province is Quebec. By population, the largest province is Ontario.
If you are asking which province has the largest population, the answer is Ontario; but if you are asking which province has the highest population density, the answer is Prince Edward Island.
The largest Canadian province in terms of population is Ontario. Based on the 2006 Statistics Canada census, the population of Ontario was 12,160,282 that year. The largest Canadian province in terms of land mass is Quebec. Taken from the 2006 census, Quebec's land area is 1,356,366.78 square kilometres. Note: Nunavut is a Canadian territory, not a province, that has a land area of 1,932,254.97 square kilometres and a population of 29,474 inhabitants in 2006.
Newfoundland and Labrador.
New Brunswick