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You cannot unlock Devil Jin in Tekken Tag Tournament, the first appearance of Devil Jin is in Tekken 4, and the first time you can use him is in Tekken 5.
You need to use Playon software and remote play from your PS3. Then connect your PSP to your Ps3.
You don't use a website, you connect the PSP to the PlayStation Network, where you can purchase and download games.
The PSP has a menu option for the PlayStation Network, simply use this and connect to wi-fi, you can purchase and download games there.
The PSP Go does not play PS3 games it plays PSPGo games If you have existing PSP games on your PS3 then you can use them