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In my opinion, it would probably have to be Mewtwo. I mean there might be harder things out there, but Mewtwo was the biggest challenge I had ever faced in Soul Silver. (NOTE: HEART GOLD AND SOUL SILVER IS BASICALLY THE SAME THINGS. THE ONLY DIFFERENCES ARE NAMES OF THE GAMES AND VERSION EXCLUSIVE POKEMON.)
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Earn +20 ptsQ: What is the hardest Pokemon to catch in Pokemon HeartGold?
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Where and how can you catch Lombre in Pokemon HeartGold?
You can catch Lombre in Pokemon HeartGold in the Safari Zone at a waterside area once you receive the National Pokedex.
How do you get mightyena in Pokemon HeartGold?
Find and then catch
Can you catch cyndaquil in HeartGold?
You can't catch it. It's a starter pokemon.
How do you catch a Venusaur on Pokemon HeartGold?
you do not catch it . you can bulbasaur when you get it from proff oak
Where can you catch growlithe in Pokemon HeartGold?
you can catch a growlithe at route 37.
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