sometime in GT.
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if I'm not mistaken its episode 280 in the uncut version and the episode is called "Vegeta's Respect"
Vegeta turns ssj4 in episode 59 of dragon-ball gt
episode 213
well goku fights in an episode called "Battle for the Universe Begins" in the uncut series it's episode 279 that they start in and if I'm not mistaken its episode 280 in the uncut version were vegeta fights buu and the episode is called "Vegeta's Respect".
episode 214 when hes majin