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Well, this is if you have Pokemon Emerald and LeafGreen AND you know how to duplicate in Emerald, then follow these steps. It'll take some time though. (You need a MasterBall in Emerald too.)

1. In Emerald, make ANY Pokemon of yours HOLD a masterball.

2. Then, duplicate that Pokemon the number of masterballs you want. (EX. I want 10 masterballs, so I duplicate it nine times. {remember, it's counting the one you already have})

3. Take the masterballs from the multiple Pokemon.

4. trade Pokemon that are holding masterballs to leafgreen.

Sorry I didn't give you UNLIMITED but that's all I have. Oh and also, don't use ALL your masterballs, then you can't duplicate any more. So I hope this helped!!
Materials:

-two Pokemon games

-two game consoles

-trading cable

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Q: How do you get unlimited masterballs in Pokemon Leaf Green?
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