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You go to Ruins of Alph in Johto and solve all four puzzles of ancient pokemon, Kabuto, Ho-oh, Aerodactyl, and Omanyte. If you solve it correctly you will fall into the Unown cave and for each puzzle you solve more unowns will appear. If you solve all the puzzles you should have unlocked all the unowns and should be able to catch all of them if you have patience.

(If you don't fall in the cave that means you haven't done the puzzle correctly)

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Q: How do you get the Unknowns in Pokemon Gold?
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