They are rare in route 7 and the safari zone
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Houndour can be found in Route 7 in SoulSilver and it can also be found in the Safari Zone.
You can find it in Pokemon Platinum, Pokemon Crystal, Pokemon HeartGold, and Pokemon SoulSilver.
You can find wild Houndour in route 7 and in the Safari Zone. From there, evolve it into Houndoom.
You can only catch him in route 7. (you can catch him also in the safari zone, but you have to have some sort of item...)
You can catch a Houndour in the Altering Cave in Pokemon FireRed.