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You should save the game right before you battle it (so if you lose, you can turn off the power and try again), use a move that blocks Mesprit from running, and use weak moves until Mesprit seems like it has 1 HP left (or u could catch a sneasel and teach it false swipe), then use a Poke-ball that seems to be the best for it. (Note:If Mesprit keeps on breaking out of the Poke-ball, then use weaker ones to try and stall it, and then use a good one. Heal Balls are better than they look.)

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Q: How do you catch mesprit easily in Pokemon diamond?
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