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Yes you could for further information go to YouTube and serch 'how to catch absol in soul silver' it should be the first thing that comes up(hope it helped)
Absol is available (but rare) at Slowpoke well,Union cave,Mt.Motar,Dark cave,Whirl islands,Mt.Silver,Ice path,The Cliff cave,Digglet's cave,Mt.Moon,Cerulean cave,Rock tunnel,Seafoam islands,Victory road and Tohjo falls.
Earliest you can catch Absol is in the Slowpoke Well.
You can either transfer it from another game e.g Emerald, or set the radio to Hoen Music when it plays on Wednesday.

You then have a 20% of catching an Absol in a cave.

It's much harder to catch it without the music playing, as it is rare, but still possible.

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