No
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I think the question is "Do you use an original Xbox or Xbox 360 controller when playing original Xbox games on an Xbox 360?" If it is than, you use an Xbox 360 controller. Left Bumper turns into "white button" Right Bumper turns into "black button"
The same way you connect it to a regular Xbox 360.
There is no way to use your existing Xbox 360 controller on your PC. However, Microsoft have released a PC controller which is a Xbox controller.
The Xbox 360 controller will not work on an original xbox console. Similarly, an original xbox controller will not work with the xbox 360. Each controller only works with its respective console. Xbox 360 Controller --> Xbox 360 Xbox controller --> Xbox
You can sync your controller into your xbox 360.To do that there are certain buttons on the controller and the xbox 360 you push to sync the controller.