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Yes, but Mewtwo is Powerful and very hard to capture even with an Ultra Ball. Best way to do this is Paralyze it, and bring it down to the red HP level.

Moves: Safeguard, Recover, Psychic & Swift

Level: 70

Location: Cerulean Cave

I suggest you take 99 Pokeballs and some high leveled Pokemon as Mewtwo is not all fun and games as its very Powerful, fast and has Fair Bulk. Be prepared and Good Luck.

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Q: Can you catch mew two with a pokeball in leafgreen?
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