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He died by a demon.
Because no one liked his character Andy and they wanted a twist with every end of each season Season 1 last episode ~ Andy Dies Season 2 Last Episode ~ Dan Moves Season 3 Last Episode ~ Prue Dies Season 4 Last Episode ~ They Get A Chance 2 be Mortal Season 5 Last Episode~ Leo Becomes an Elder and has 2 leave the charmed 1s Season 6 Last Episode ~ Chris Dies Season 7 Last Episode ~ Charmed Ones Fake Own Death Season 8 Last Episode ~ Piper goes back in time 2 save phoebe and Paige and they get Leo back
The first main character to die in Charmed was Andy (Prue's boyfriend). But out of the sisters Prue was the first to die
He left because he didn't get along with Shannen Doherty (Prue).
Season 1 episode 22 Deja Vu All Over Again