Jiraiya trains Naruto in many episodes. Jiraiya is Naruto's new trainer instead of Kakashi sensei. But Jiraiya starts training him in episode #53 and just becomes Naruto's new trainer, also, Jiraiya is one of the three legendary sannin along with Tsunade and Orochimaru.
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The episode of Naruto when Jiraya dies is in the 133rd episode of the series. The name of the episode was The Tale of Jiraiya.
Naruto end of episode 56 and start of episode 57
That would be in episode 35.
Naruto shippuden episode 128 Jiraiya ninja scroll part two
lol the question says what episode does jiraiya and tsunade fight orochimaru, and its 52 not 133, 133 when naruto and sasuke fought